Screwtape2
Blue Crack Addict
Carrey based his performance in Forever off of Gorshin. I like him in that movie, too, but any of the '60s Batman villains top the Burton/Schumacher villains in a landslide. Yes, even Cesar Romero over Jack Nicholson.
I think it is all a matter of perspective. Personally, I think Batman Begins is only live action Batman interpretation that matched the feel of the comics in terms of the villians.
Actually most superhero films don't capture the true essence of the villians.